Multiline Laser Interferometry for Non-Contact Dynamic Morphing of Hierarchical Surfaces

Hierarchical surface structuring is a critical aspect of advanced materials design, impacting fields ranging from optics to biomimetics. Among several laser-based methods for complex structuring of photo-responsive surfaces, the broadband vectorial interferometry proposed here offers unique performances. Such a method leverages a polychromatic laser source, an unconventional choice for holographic encoding, to achieve deterministic multiscale surface structuring through interference light patterning. Azopolymer films are used as photosensitive substrates. By exploring the interaction between optomechanical stress modulations at different spatial periodicities induced within the polymer bulk, we demonstrate the emergence of hierarchical Fourier surfaces composed of multiple deterministic levels. These structures range from sub-micrometer to tens of micrometers scale, exhibiting a high degree of control over their morphology. The experimental findings reveal that the optical encoding scheme significantly influences the resulting topographies. The polarization light patterns lead to more regular and symmetric hierarchical structures compared to those obtained with intensity patterns, underscoring the role of vectorial light properties in controlling surface morphologies. The proposed method is fully scalable, compatible with more complex recording schemes (including multi-beam interference), and it is applicable to a wide range of advanced technological fields. These include optics and photonics (diffractive elements, polarimetric devices), biomimetic surfaces, topographical design, information encoding, and anti-counterfeiting, offering a rapid, reliable, and versatile strategy for high-precision surface structuring at a submicrometric scale.